TY - JOUR
T1 - A model dielectric function for low and very high momentum transfer
AU - Vos, Maarten
N1 - Publisher Copyright:
© 2015 Elsevier B.V. All rights reserved.
PY - 2016/1/1
Y1 - 2016/1/1
N2 - A model dielectric function is derived for TiO2 based on reflection electron energy loss spectroscopy data and photoabsorption cross sections. The model is based on a set of Mermin oscillators. The input data is dominated by excitations at low momentum transfer, i.e. near the optical limit. Surprisingly the dielectric function derived at low momentum transfer describes the Compton profile quite well, while approaches based on Drude oscillators fail dramatically. The link between the dielectric function in the high-momentum transfer limit and a Compton profile is discussed. The underlying reason why the Mermin approach, which is based on a free electron model, is successful in describing the Compton profile is tentatively discussed.
AB - A model dielectric function is derived for TiO2 based on reflection electron energy loss spectroscopy data and photoabsorption cross sections. The model is based on a set of Mermin oscillators. The input data is dominated by excitations at low momentum transfer, i.e. near the optical limit. Surprisingly the dielectric function derived at low momentum transfer describes the Compton profile quite well, while approaches based on Drude oscillators fail dramatically. The link between the dielectric function in the high-momentum transfer limit and a Compton profile is discussed. The underlying reason why the Mermin approach, which is based on a free electron model, is successful in describing the Compton profile is tentatively discussed.
KW - Compton profile
KW - Mermin dielectric function
KW - Reflection electron energy loss spectroscopy
UR - http://www.scopus.com/inward/record.url?scp=84944345466&partnerID=8YFLogxK
U2 - 10.1016/j.nimb.2015.09.091
DO - 10.1016/j.nimb.2015.09.091
M3 - Article
SN - 0168-583X
VL - 366
SP - 6
EP - 12
JO - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
JF - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
ER -