Abstract
We report on a study of the dynamics of a recently discovered light-induced, surface-assisted, structural phase transition from a common orthorhombic phase of α-gallium to a highly reflective phase that occurs at temperatures just below the metal's bulk melting point (30°C). It is fully reversible with dynamics occurring on a nanosecond/microsecond time scale and can be stimulated by very low-intensity radiation, typically approx. 10-5 W/μm2. The two gallium phases involved have significantly different optical properties and this difference gives rise to a gigantic optical nonlinearity, χ(3) approx. 1 esu, that offers tremendous new opportunities for controlling light with light. The microscopic model of the effect is discussed.
Original language | English |
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Pages (from-to) | 646-648 |
Number of pages | 3 |
Journal | Journal of Luminescence |
Volume | 87 |
DOIs | |
Publication status | Published - May 2000 |
Event | International Conference on Luminescence and Optical Spectroscopy of Condensed Matter (ICL'99) - Osaka, Jpn Duration: 23 Aug 1999 → 27 Aug 1999 |