Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond

K. M.C. Fu, C. Santori, P. E. Barclay, L. J. Rogers, N. B. Manson, R. G. Beausoleil

    Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

    1 Citation (Scopus)

    Abstract

    The understanding of the coherence properties of photons emitted from negatively charged nitrogen-vacancy (NV) centers in diamond is essential for the success of quantum information applications based on indistinguishable photons. Here we study both the polarization of photons emitted from and the linewidth of photons absorbed by single NV centers as a function of temperature T. We find that for T < 100 K the main dephasing mechanism contributing to the linewidth broadening is phonon-mediated population transfer between the two excited orbital states. The observed T5 temperature dependence of the population transfer rate and linewidth is experimental evidence of a dynamic Jahn-Teller effect in the excited states.

    Original languageEnglish
    Title of host publicationAdvances in Photonics of Quantum Computing, Memory, and Communication III
    DOIs
    Publication statusPublished - 2010
    EventAdvances in Photonics of Quantum Computing, Memory, and Communication III - San Francisco, CA, United States
    Duration: 27 Jan 201028 Jan 2010

    Publication series

    NameProceedings of SPIE - The International Society for Optical Engineering
    Volume7611
    ISSN (Print)0277-786X

    Conference

    ConferenceAdvances in Photonics of Quantum Computing, Memory, and Communication III
    Country/TerritoryUnited States
    CitySan Francisco, CA
    Period27/01/1028/01/10

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