Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond

Kai Mei C. Fu; Charles Santori; Paul E. Barclay; Lachlan J. Rogers; Neil B. Manson; Raymond G. Beausoleil

doi:10.1103/PhysRevLett.103.256404

Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond

Kai Mei C. Fu, Charles Santori, Paul E. Barclay, Lachlan J. Rogers, Neil B. Manson, Raymond G. Beausoleil

Research output: Contribution to journal › Article › peer-review

236 Citations (Scopus)

Abstract

The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T5 dependence for T<100K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.

Original language	English
Article number	256404
Journal	Physical Review Letters
Volume	103
Issue number	25
DOIs	https://doi.org/10.1103/PhysRevLett.103.256404
Publication status	Published - 17 Dec 2009

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10.1103/PhysRevLett.103.256404

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abstract = "The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T5 dependence for T<100K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.",

author = "Fu, \{Kai Mei C.\} and Charles Santori and Barclay, \{Paul E.\} and Rogers, \{Lachlan J.\} and Manson, \{Neil B.\} and Beausoleil, \{Raymond G.\}",

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AU - Fu, Kai Mei C.

AU - Santori, Charles

AU - Barclay, Paul E.

AU - Rogers, Lachlan J.

AU - Manson, Neil B.

AU - Beausoleil, Raymond G.

PY - 2009/12/17

Y1 - 2009/12/17

N2 - The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T5 dependence for T<100K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.

AB - The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T5 dependence for T<100K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.

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DO - 10.1103/PhysRevLett.103.256404

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Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond

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