Recoil-ion momentum distributions for two-photon double ionization of He and Ne by 44 eV free-electron laser radiation

A. Rudenko*, L. Foucar, M. Kurka, Th Ergler, K. U. Kühnel, Y. H. Jiang, A. Voitkiv, B. Najjari, A. Kheifets, S. Lüdemann, T. Havermeier, M. Smolarski, S. Schössler, K. Cole, M. Schöffler, R. Dörner, S. Düsterer, W. Li, B. Keitel, R. TreuschM. Gensch, C. D. Schröter, R. Moshammer, J. Ullrich

*Corresponding author for this work

    Research output: Contribution to journalArticlepeer-review

    138 Citations (Scopus)

    Abstract

    Recoil-ion momentum distributions for two-photon double ionization of He and Ne (ω=44eV) have been recorded with a reaction microscope at FLASH (the free-electron laser at Hamburg) at an intensity of ∼1×1014W/cm2 exploring the dynamics of the two fundamental two-photon-two-electron reaction pathways, namely, sequential and direct (or nonsequential) absorption of the photons. We find strong differences in the recoil-ion momentum patterns for the two mechanisms pointing to the significantly different two-electron emission dynamics and thus provide serious constraints for theoretical models.

    Original languageEnglish
    Article number073003
    JournalPhysical Review Letters
    Volume101
    Issue number7
    DOIs
    Publication statusPublished - 15 Aug 2008

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