TY - JOUR
T1 - Resonance-Amplified Terahertz Near-Field Spectroscopy of a Single Nanowire
AU - Norman, Sarah
AU - Chu, Greg
AU - Peng, Kun
AU - Seddon, James
AU - Hale, Lucy L.
AU - Tan, Hark Hoe
AU - Jagadish, Chennupati
AU - Mouthaan, Ralf
AU - Alexander-Webber, Jack
AU - Joyce, Hannah J.
AU - Johnston, Michael B.
AU - Mitrofanov, Oleg
AU - Siday, Thomas
N1 - Publisher Copyright:
© 2024 The Authors. Published by American Chemical Society.
PY - 2024/12/11
Y1 - 2024/12/11
N2 - Nanoscale material systems are central to next-generation optoelectronic and quantum technologies, yet their development remains hindered by limited characterization tools, particularly at terahertz (THz) frequencies. Far-field THz spectroscopy techniques lack the sensitivity for investigating individual nanoscale systems, whereas in near-field THz nanoscopy, surface states, disorder, and sample-tip interactions often mask the response of the entire nanoscale system. Here, we present a THz resonance-amplified near-field spectroscopy technique that can detect subtle conductivity changes in isolated nanoscale systems─such as a single InAs nanowire─under ultrafast photoexcitation. By exploiting the spatial localization and resonant field enhancement in the gap of a bowtie antenna, our approach enables precise measurements of the nanostructures through shifts in the antenna resonant frequency, offering a direct means of extracting the system response, and unlocking investigations of ultrafast charge-carrier dynamics in isolated nanoscale and microscale systems.
AB - Nanoscale material systems are central to next-generation optoelectronic and quantum technologies, yet their development remains hindered by limited characterization tools, particularly at terahertz (THz) frequencies. Far-field THz spectroscopy techniques lack the sensitivity for investigating individual nanoscale systems, whereas in near-field THz nanoscopy, surface states, disorder, and sample-tip interactions often mask the response of the entire nanoscale system. Here, we present a THz resonance-amplified near-field spectroscopy technique that can detect subtle conductivity changes in isolated nanoscale systems─such as a single InAs nanowire─under ultrafast photoexcitation. By exploiting the spatial localization and resonant field enhancement in the gap of a bowtie antenna, our approach enables precise measurements of the nanostructures through shifts in the antenna resonant frequency, offering a direct means of extracting the system response, and unlocking investigations of ultrafast charge-carrier dynamics in isolated nanoscale and microscale systems.
KW - Nanowires
KW - Near-field microscopy
KW - Terahertz spectroscopy
KW - Ultrafast dynamics
UR - http://www.scopus.com/inward/record.url?scp=85210275658&partnerID=8YFLogxK
U2 - 10.1021/acs.nanolett.4c04395
DO - 10.1021/acs.nanolett.4c04395
M3 - Article
C2 - 39588607
AN - SCOPUS:85210275658
SN - 1530-6984
VL - 24
SP - 15716
EP - 15723
JO - Nano Letters
JF - Nano Letters
IS - 49
ER -