Rydberg states of silver: Excitation dynamics of doped helium droplets

F. Federmann, K. Hoffmann, N. Quaas, J. D. Close

    Research output: Contribution to journalArticlepeer-review

    35 Citations (Scopus)

    Abstract

    Silver atoms, initially embedded in nanodroplets of superfluid helium (roughly 104 atoms in size), are found to move to the surface and desorb when excited to the broadened 5p level. The absorption of a second photon within less than 10 ns leads to the population of previously unobserved Rydberg states (20 < n < 60) of free silver atoms. This is the first result showing laser induced movement of a foreign atom from the inside to the surface of a nanodroplet of superfluid helium.

    Original languageEnglish
    Pages (from-to)2548-2551
    Number of pages4
    JournalPhysical Review Letters
    Volume83
    Issue number13
    DOIs
    Publication statusPublished - 1 Jan 1999

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