Stimulated Rayleigh-Bragg scattering in two-photon absorbing media

Guang S. He*, Changgui Lu, Qingdong Zheng, Paras N. Prasad, Petros Zerom, Robert W. Boyd, Marek Samoc

*Corresponding author for this work

    Research output: Contribution to journalArticlepeer-review

    26 Citations (Scopus)

    Abstract

    The origin and mechanism of backward stimulated Rayleigh scattering in two-photon absorbing media are studied theoretically and experimentally. This type of stimulated scattering has the unusual features of no frequency shift and low pump threshold requirement compared to all other known stimulated scattering effects. This frequency-unshifted stimulated Rayleigh scattering effect can be well explained by a two-photon-excitation-enhanced Bragg grating reflection model. The reflection of the forward pump beam from this stationary Bragg grating may substantially enhance the backward Rayleigh scattering beam, providing a positive feedback mechanism without causing any frequency shift. A two-counterpropagating-beam-formed grating experiment in a two-photon absorbing dye solution is conducted. The measured dynamic behavior of Bragg grating formation and reflectivity properties are basically consistent with the predictions from the proposed model.

    Original languageEnglish
    Article number063810
    JournalPhysical Review A - Atomic, Molecular, and Optical Physics
    Volume71
    Issue number6
    DOIs
    Publication statusPublished - Jun 2005

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