The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet

Rizwan Nabi; Ben Atkinson; Jakob Staab; Jonathan Skelton; Nicholas F Chilton

doi:10.1039/D4CC03768E

The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet

Rizwan Nabi, Ben Atkinson, Jakob Staab, Jonathan Skelton, Nicholas F Chilton

Research School of Chemistry

Research output: Contribution to journal › Article › peer-review

Abstract

Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that... Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that agree with experiment. They show that low-energy phonon scattering is a significant contribution to the high-performance of dysprosocenium SMMs.

Original language	English
Number of pages	4
Journal	Chemical Communications
DOIs	https://doi.org/10.1039/D4CC03768E
Publication status	Published - 2024

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http://pubs.rsc.org/en/Content/ArticleLanding/2024/CC/D4CC03768E

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title = "The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet",

abstract = "Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that... Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that agree with experiment. They show that low-energy phonon scattering is a significant contribution to the high-performance of dysprosocenium SMMs.",

author = "Rizwan Nabi and Ben Atkinson and Jakob Staab and Jonathan Skelton and Chilton, {Nicholas F}",

year = "2024",

doi = "10.1039/D4CC03768E",

language = "English",

journal = "Chemical Communications",

issn = "1359-7345",

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T1 - The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet

AU - Nabi, Rizwan

AU - Atkinson, Ben

AU - Staab, Jakob

AU - Skelton, Jonathan

AU - Chilton, Nicholas F

PY - 2024

Y1 - 2024

N2 - Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that... Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that agree with experiment. They show that low-energy phonon scattering is a significant contribution to the high-performance of dysprosocenium SMMs.

AB - Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that... Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that agree with experiment. They show that low-energy phonon scattering is a significant contribution to the high-performance of dysprosocenium SMMs.

U2 - 10.1039/D4CC03768E

DO - 10.1039/D4CC03768E

M3 - Article

SN - 1359-7345

JO - Chemical Communications

JF - Chemical Communications

ER -

The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet

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