TY - JOUR
T1 - Thermally Driven Transport and Relaxation Switching Self-Powered Electromagnetic Energy Conversion
AU - Cao, Maosheng
AU - Wang, Xixi
AU - Cao, Wenqiang
AU - Fang, Xiaoyong
AU - Wen, Bo
AU - Yuan, Jie
N1 - Publisher Copyright:
© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
PY - 2018/7/19
Y1 - 2018/7/19
N2 - Electromagnetic energy radiation is becoming a “health-killer” of living bodies, especially around industrial transformer substation and electricity pylon. Harvesting, converting, and storing waste energy for recycling are considered the ideal ways to control electromagnetic radiation. However, heat-generation and temperature-rising with performance degradation remain big problems. Herein, graphene-silica xerogel is dissected hierarchically from functions to “genes,” thermally driven relaxation and charge transport, experimentally and theoretically, demonstrating a competitive synergy on energy conversion. A generic approach of “material genes sequencing” is proposed, tactfully transforming the negative effects of heat energy to superiority for switching self-powered and self-circulated electromagnetic devices, beneficial for waste energy harvesting, conversion, and storage. Graphene networks with “well-sequencing genes” (w = Pc/Pp > 0.2) can serve as nanogenerators, thermally promoting electromagnetic wave absorption by 250%, with broadened bandwidth covering the whole investigated frequency. This finding of nonionic energy conversion opens up an unexpected horizon for converting, storing, and reusing waste electromagnetic energy, providing the most promising way for governing electromagnetic pollution with self-powered and self-circulated electromagnetic devices.
AB - Electromagnetic energy radiation is becoming a “health-killer” of living bodies, especially around industrial transformer substation and electricity pylon. Harvesting, converting, and storing waste energy for recycling are considered the ideal ways to control electromagnetic radiation. However, heat-generation and temperature-rising with performance degradation remain big problems. Herein, graphene-silica xerogel is dissected hierarchically from functions to “genes,” thermally driven relaxation and charge transport, experimentally and theoretically, demonstrating a competitive synergy on energy conversion. A generic approach of “material genes sequencing” is proposed, tactfully transforming the negative effects of heat energy to superiority for switching self-powered and self-circulated electromagnetic devices, beneficial for waste energy harvesting, conversion, and storage. Graphene networks with “well-sequencing genes” (w = Pc/Pp > 0.2) can serve as nanogenerators, thermally promoting electromagnetic wave absorption by 250%, with broadened bandwidth covering the whole investigated frequency. This finding of nonionic energy conversion opens up an unexpected horizon for converting, storing, and reusing waste electromagnetic energy, providing the most promising way for governing electromagnetic pollution with self-powered and self-circulated electromagnetic devices.
KW - charge transport
KW - electromagnetic energy conversion
KW - graphene
KW - relaxation
KW - self-power
UR - http://www.scopus.com/inward/record.url?scp=85050121714&partnerID=8YFLogxK
U2 - 10.1002/smll.201800987
DO - 10.1002/smll.201800987
M3 - Article
SN - 1613-6810
VL - 14
JO - Small
JF - Small
IS - 29
M1 - 1800987
ER -