Two-photon and three-photon absorption in an organometallic dendrimer

Marek Samoc; Joseph P. Morrall; Gulliver T. Dalton; Marie P. Cifuentes; Mark G. Humphrey

doi:10.1002/anie.200602341

Two-photon and three-photon absorption in an organometallic dendrimer

Marek Samoc^*, Joseph P. Morrall, Gulliver T. Dalton, Marie P. Cifuentes, Mark G. Humphrey

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

123 Citations (Scopus)

Abstract

Three at a time: The wavelength dependence of nonlinear absorption and non-linear refraction of a peripherally nitrophenylethynyl-functionalized first-generation arylethynylruthenium dendrimer (see picture; dppe = 1,2-bis(diphenylphosphanyl)ethane) was examined in the range 625-1500 nm by employing fs pulses. The compound is a strong two-photon absorber in the range 600-800 nm and an exceptional three-photon absorber in the range 1100-1200 nm. (Chemical Equation Presented).

Original language	English
Pages (from-to)	731-733
Number of pages	3
Journal	Angewandte Chemie - International Edition
Volume	46
Issue number	5
DOIs	https://doi.org/10.1002/anie.200602341
Publication status	Published - 2007

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abstract = "Three at a time: The wavelength dependence of nonlinear absorption and non-linear refraction of a peripherally nitrophenylethynyl-functionalized first-generation arylethynylruthenium dendrimer (see picture; dppe = 1,2-bis(diphenylphosphanyl)ethane) was examined in the range 625-1500 nm by employing fs pulses. The compound is a strong two-photon absorber in the range 600-800 nm and an exceptional three-photon absorber in the range 1100-1200 nm. (Chemical Equation Presented).",

keywords = "Absorption, Alkynyl ligands, Dendrimers, Nonlinear optics, Ruthenium",

author = "Marek Samoc and Morrall, {Joseph P.} and Dalton, {Gulliver T.} and Cifuentes, {Marie P.} and Humphrey, {Mark G.}",

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AU - Morrall, Joseph P.

AU - Dalton, Gulliver T.

AU - Cifuentes, Marie P.

AU - Humphrey, Mark G.

PY - 2007

Y1 - 2007

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AB - Three at a time: The wavelength dependence of nonlinear absorption and non-linear refraction of a peripherally nitrophenylethynyl-functionalized first-generation arylethynylruthenium dendrimer (see picture; dppe = 1,2-bis(diphenylphosphanyl)ethane) was examined in the range 625-1500 nm by employing fs pulses. The compound is a strong two-photon absorber in the range 600-800 nm and an exceptional three-photon absorber in the range 1100-1200 nm. (Chemical Equation Presented).

KW - Absorption

KW - Alkynyl ligands

KW - Dendrimers

KW - Nonlinear optics

KW - Ruthenium

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JO - Angewandte Chemie - International Edition

JF - Angewandte Chemie - International Edition

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ER -

Two-photon and three-photon absorption in an organometallic dendrimer

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